By Applerocks, 18 September, 2018 Forum macOS and Mac Apps does any one know if I can delete a album from my I tunes music liblibarryyyy Options Log in or register to post comments Comments iTunes If you mean PC Window 10. On iTumes go to music, artist or album select the album or artist, use application and f10 and go up to delete. You will get message asking you if you want to delete from library. Yes. It will delete from iTunes and iCloud.